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PM2.5 mass, chemical composition, and light extinction before and during the 2008 Beijing Olympics
Li, Xinghua1; He, Kebin2; Li, Chengcai3; Yang, Fumo4; Zhao, Qing2; Ma, Yongliang2; Cheng, Yuan2; Ouyang, Wenjuan4; Chen, Gangcai5
2013-11-16
摘要Distinct contrast of air quality and visibility before and during the 2008 Beijing Olympic Games provides a rare opportunity to investigate the links between PM2.5 mass, chemical composition, and light extinction in this megacity. Twenty-four hour integrated PM2.5 samples were collected, and light scattering coefficients and the concentrations of black carbon were measured at urban Beijing for this purpose during a measurement campaign from 1 July to 20 September 2008, which was classed into four stages according to the levels of emission control measures. Daily PM2.5 concentrations ranged from 15.9 to 156.7 mu g m(-3) with an average of 66.0 +/- 35.1 mu g m(-3). The average PM2.5 mass during the Olympics decreased by 49% from the second stage (20 July to 7 August), mainly due to the reduction of secondary inorganic aerosols (i.e., sulfate, nitrate, and ammonium (SNA)). The counterintuitive increase of PM2.5 mass (by 27% on average) during the second stage with two most serious haze episodes, although more rigorous emission control measures were in place, compared to the first stage (1-19 July), was mainly explained by the unfavorable meteorology and input of sulfate aerosols. A daily PM2.5 mass threshold of 50 mu g m(-3) was extracted for frequent haze occurrence. The extinction fractions of SNA and organic material were each approximately 30% during the 20% best visibility days but changed to 81.7% and 8.4%, respectively, during the 20% worst visibility days. The results indicated that the role of SNA was magnified in haze formation during the 2008 summer in Beijing.
DOI10.1002/2013JD020106
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发表期刊JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES
ISSN2169-897X
卷号118期号:21页码:12158-12167
通讯作者Yang, FM (reprint author), Chinese Acad Sci, Chongqing Inst Green & Intelligent Technol, Key Lab Reservoir Aquat Environm, Chongqing 401122, Peoples R China.
收录类别SCI
WOS记录号WOS:000330611800018
语种英语