中国科学院重庆绿色智能技术研究院机构知识库

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	H2O2-free photo-Fenton system for antibiotics degradation in water via the synergism of oxygen-enriched graphitic carbon nitride polymer and nano manganese ferrite
	Yi, Huan1,2,3; Lai, Cui1,2; Huo, Xiuqin1,2; Qin, Lei1,2; Fu, Yukui1,2; Liu, Shiyu1,2; Li, Ling1,2; Zhang, Mingming1,2; Chen, Ming3; Zeng, Guangming1,2
	2022-01-06
摘要	The use of antibiotics in human beings is a most significant milestone in the present era. However, owing to the chemical diversity and complexity, antibiotic removal from water has been an issue with the massive emission. As an efficient technology for antibiotic wastewater treatment, photo-Fenton oxidation has drawn much attention. In this work, we constructed a photo-Fenton system by combining oxygen-enriched graphitic carbon nitride polymer (OCN) and manganese ferrite (MnFe2O4) to form OCN-MnFe2O4 (OMF) composites, which show good performance for antibiotics degradation without adding H2O2. The degradation efficiency within 1 h for tetracycline, oxytetracycline and ciprofloxacin were 86.5%, 82.2% and 42.7%, respectively. Both radical pathways (PFRs, OH, O-2(-) and h(+)) and non-radical pathways (electron transfer and O-1(2)) play roles in antibiotic degradation. Additionally, the performance of this photo-Fenton system over OMF was nearly not affected by water matrix and inorganic salt ions, exhibiting high stability. It is anticipated that this photo-Fenton system is highly efficient for the treatment of antibiotics-polluted water.
DOI	10.1039/d1en00869b
发表期刊	ENVIRONMENTAL SCIENCE-NANO
ISSN	2051-8153
页码	12
通讯作者	Chen, Ming(chenming@cigit.ac.cn) ; Zeng, Guangming(zgming@hnu.edu.cn)
收录类别	SCI
WOS记录号	WOS:000744615300001
语种	英语